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Answer for the clue "Loosens, as some shirts ", 9 letters:
unbuttons

Word definitions for unbuttons in dictionaries

Wiktionary Word definitions in Wiktionary
vb. (en-third-person singular of: unbutton )

Usage examples of unbuttons.

She unbuttons the yellow suit jacket, only then realizing that there aren’t any hangers in the shallow closet by the door.

I am amused by the way she leers at me through her tears as she expertly unbuttons my trouser buttons and unzips me.

Michell drops her blouse on the floor next to his jacket and unbuttons her skirt.