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Douglas Harper's Etymology Dictionary
over-populate

also overpopulate, "to overrun with too many people," 1828 (implied in overpopulated), from over- + populate (v.). Related: Overpopulating. Over-populous "over-populated" is attested from 1670s.

Usage examples of "over-populate".

It is hardly to be wondered at that we live on an over-populated globe, when mankind continually populates the deserts, the deeps, the interior of the Earth, and the Heavens, with a riotous assembly of imaginary beings.

The more people he can remove from the over-populated country and place in positions of influence overseas, the better the potential to achieve international power bases working under directives from the mother country.