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Alcalalí (, ) is a Valencian municipality in the comarca of Marina Alta, province of Alicante, Spain.

It is situated in the Pop Valley (Vall de Pop) between the Serra del Ferrer and the mounts of Segili. It is bordered by Pedreguer and Benidoleig to the north, Jalón and Llíber to the east; Orba, Murla, Benigembla and Parcent to the west and Tàrbena to the south.